Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)

Russell Cooper; Igor Rahinov; Cheng Yuan; Xueming Yang; Daniel J. Auerbach; Alec M. Wodtke

doi:10.1116/1.3071971

Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)

Russell Cooper, Igor Rahinov, Cheng Yuan, Xueming Yang, Daniel J. Auerbach, Alec M. Wodtke

Research output: Contribution to journal › Article › peer-review

Abstract

The authors report high resolution state resolved measurements of the translational inelasticity of HCl (v=0→0,J=0→4) colliding with a Au(111) surface at near normal incidence in the energy range of 0.28-1.27 eV. The translational inelasticity is large and indistinguishable from previous measurements for the HCl (v=2→2,J=1→5) channel. They discuss these observations in terms of an impulse approximation as well as the possible role of translational excitation of electron-hole pairs in the solid.

Original language	English
Pages (from-to)	907-912
Number of pages	6
Journal	Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films
Volume	27
Issue number	4
DOIs	https://doi.org/10.1116/1.3071971
State	Published - 2009
Externally published	Yes

Bibliographical note

Funding Information:
The authors gratefully acknowledge the financial support from the Department of Energy Office of Basic Energy Sciences, under Grant No. DE-FG02-03ER15441 as well as the Partnership for International Research and Education—for Electronic Chemistry and Catalysis at Interfaces—NSF Grant No. OISE-0530268.

Access to Document

10.1116/1.3071971

Cite this

Cooper, R., Rahinov, I., Yuan, C., Yang, X., Auerbach, D. J., & Wodtke, A. M. (2009). Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111). Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films, 27(4), 907-912. https://doi.org/10.1116/1.3071971

@article{6cfe485729d04d9584223081e4fb80cd,

title = "Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)",

abstract = "The authors report high resolution state resolved measurements of the translational inelasticity of HCl (v=0→0,J=0→4) colliding with a Au(111) surface at near normal incidence in the energy range of 0.28-1.27 eV. The translational inelasticity is large and indistinguishable from previous measurements for the HCl (v=2→2,J=1→5) channel. They discuss these observations in terms of an impulse approximation as well as the possible role of translational excitation of electron-hole pairs in the solid.",

author = "Russell Cooper and Igor Rahinov and Cheng Yuan and Xueming Yang and Auerbach, \{Daniel J.\} and Wodtke, \{Alec M.\}",

year = "2009",

doi = "10.1116/1.3071971",

language = "אנגלית",

volume = "27",

pages = "907--912",

journal = "Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films",

issn = "0734-2101",

publisher = "AVS Science and Technology Society",

number = "4",

}

Cooper, R, Rahinov, I, Yuan, C, Yang, X, Auerbach, DJ & Wodtke, AM 2009, 'Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)', Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films, vol. 27, no. 4, pp. 907-912. https://doi.org/10.1116/1.3071971

Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111). / Cooper, Russell; Rahinov, Igor; Yuan, Cheng et al.
In: Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films, Vol. 27, No. 4, 2009, p. 907-912.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Efficient translational excitation of a solid metal surface

T2 - State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)

AU - Cooper, Russell

AU - Rahinov, Igor

AU - Yuan, Cheng

AU - Yang, Xueming

AU - Auerbach, Daniel J.

AU - Wodtke, Alec M.

PY - 2009

Y1 - 2009

N2 - The authors report high resolution state resolved measurements of the translational inelasticity of HCl (v=0→0,J=0→4) colliding with a Au(111) surface at near normal incidence in the energy range of 0.28-1.27 eV. The translational inelasticity is large and indistinguishable from previous measurements for the HCl (v=2→2,J=1→5) channel. They discuss these observations in terms of an impulse approximation as well as the possible role of translational excitation of electron-hole pairs in the solid.

AB - The authors report high resolution state resolved measurements of the translational inelasticity of HCl (v=0→0,J=0→4) colliding with a Au(111) surface at near normal incidence in the energy range of 0.28-1.27 eV. The translational inelasticity is large and indistinguishable from previous measurements for the HCl (v=2→2,J=1→5) channel. They discuss these observations in terms of an impulse approximation as well as the possible role of translational excitation of electron-hole pairs in the solid.

UR - https://www.scopus.com/pages/publications/67650321320

U2 - 10.1116/1.3071971

DO - 10.1116/1.3071971

M3 - ???researchoutput.researchoutputtypes.contributiontojournal.article???

AN - SCOPUS:67650321320

SN - 0734-2101

VL - 27

SP - 907

EP - 912

JO - Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films

JF - Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films

IS - 4

ER -

Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)

Abstract

Bibliographical note

Access to Document

Other files and links

Fingerprint

Cite this